According to the characteristics of spacecraft capturing noncooperative targets in orbit, an increment feedback controller based on nonlinear iterative sliding mode is presented. Firstly, the attitude tracking error equation is established, and then, an increment feedback control law based on bounded iterative sliding modes is proposed, which does not need to estimate the uncertain moment of inertia and external disturbances. For comparing, an adaptive sliding mode controller has been designed in the paper. Some numerical simulations have been given in the presence of spacecraft on-orbit capturing noncooperative target, and the simulation results show that the increment feedback controller has strong robustness to the unknown parametric variations and external disturbances and has a smaller control input torque in control process.